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@ARTICLE{Lange:284943,
author = {P. F. Lange and O. Schilling$^*$ and P. F. Huesgen},
title = {{P}ositional proteomics: is the technology ready to study
clinical cohorts?},
journal = {Expert review of proteomics},
volume = {20},
number = {12},
issn = {1478-9450},
address = {Abingdon},
publisher = {Taylor $\&$ Francis Group},
reportid = {DKFZ-2023-02143},
pages = {309-318},
year = {2023},
note = {2023 Jul-Dec;20(12):309-318},
abstract = {Positional proteomics provides proteome-wide information on
protein termini and their modifications, uniquely enabling
unambiguous identification of site-specific, limited
proteolysis. Such proteolytic cleavage irreversibly modifies
protein sequences resulting in new proteoforms with distinct
protease-generated neo-N and C-termini and altered
localization, activity. Mis regulated proteolysis is
implicated in a wide variety of human diseases. Protein
termini, therefore, constitute a huge, largely unexplored
source of specific analytes that provides a deep view into
the functional proteome and a treasure trove for
biomarkers.We briefly review principal approaches to define
protein termini and discuss recent advances in method
development. We further highlight the potential of
positional proteomics to identify and trace specific
proteoforms, with a focus on proteolytic processes altered
in disease. Lastly, we discuss current challenges and
potential for applying positional proteomics in biomarker
and pre-clinical research.Recent developments in positional
proteomics have provided significant advances in sensitivity
and throughput. In-depth analysis of proteolytic processes
in clinical cohorts thus appears feasible in the near
future. We argue that this will provide insights into the
functional state of the proteome and offer new opportunities
to utilize proteolytic processes altered or targeted in
disease as specific diagnostic, prognostic and companion
biomarkers.},
keywords = {HUNTER (Other) / Positional proteomics (Other) / biomarker
(Other) / degradomics (Other) / proteoform (Other) /
proteolysis (Other) / terminomics (Other)},
cin = {FR01},
ddc = {610},
cid = {I:(DE-He78)FR01-20160331},
pnm = {899 - ohne Topic (POF4-899)},
pid = {G:(DE-HGF)POF4-899},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:37869791},
doi = {10.1080/14789450.2023.2272046},
url = {https://inrepo02.dkfz.de/record/284943},
}