% IMPORTANT: The following is UTF-8 encoded. This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.
@ARTICLE{Rashidipour:294828,
author = {M. Rashidipour and S. Abbaszadeh and M. Birjandi and N.
Pajouhi and S. Ahmadi Somaghian and G. Goudarzi and S.
Shahryarhesami$^*$ and M. Moradi Sarabi and E. Babaeenezhad},
title = {{A}ntimicrobial activity and cytotoxic and epigenetic
effects of tannic acid-loaded chitosan nanoparticles.},
journal = {Scientific reports},
volume = {14},
number = {1},
issn = {2045-2322},
address = {[London]},
publisher = {Macmillan Publishers Limited, part of Springer Nature},
reportid = {DKFZ-2024-02539},
pages = {30405},
year = {2024},
abstract = {Tannic acid (TA) is a potent antitumor agent, but its low
bioavailability and absorption limit its use. In this study,
it was loaded into chitosan-based nanoparticles (Chi-NPs) to
overcome these limitations and to improve its antimicrobial
and anticancer activities. TA-loaded Chi-NPs (Chi-TA-NPs)
were synthesized using the ionic gelation method and
physicochemically characterized by FE-SEM, FTIR, XRD, PDI,
DLS, and zeta potential analysis. Additionally, the
antimicrobial activity of Chi-TA-NPs against two G+
bacterial strains, two G- bacterial strains, and a fungal
strain (Candida albicans) was investigated using the
microbroth dilution method. MTT assay was used to examine
the cytotoxic effects of Chi-TA-NPs on HepG2 cells. The
expression of DNA methyltransferase 1 (DNMT1), DNMT3A, and
DNMT3B was examined in HepG2 cells using RT-qPCR. The amount
of 5-methylcytosine in the HepG2 cell-derived genomic DNA
was measured using ELISA. FE-SEM micrographs showed the
loading of TA into the chitosan-based formulation. The peaks
detected in the XRD and FTIR analyses confirmed the
formation of the Chi-TA-NPs. The PDI value (0.247 ± 0.03),
size (567.0 ± 25.84 nm), and zeta potential (17.0 ± 5.86
mV) confirmed the relative stability of Chi-TA-NPs. A
constant release profile in line with the Korsmeyer-Peppas
model was detected for Chi-TA-NPs, such that approximately
$44\%$ of TA was released after 300 min. In addition,
Chi-TA-NPs exhibited effective antimicrobial activity
against the studied microbial strains, as manifested by MIC
values ranging from 250 to 1000 µg/mL. Chi-TA-NPs induced
cytotoxicity in liver tumor cell line, with an IC50 value of
500 µg/mL. Furthermore, Chi-TA-NPs considerably decreased
the expression of DNMT1 (2.52-fold; p = 0.01), DNMT3A
(2.96-fold; p = 0.004), and DNMT3B (2.94-fold; p < 0.0001).
However, 5-methylcytosine levels in HepG2 cells were
unaffected by Chi-TA-NPs treatment (p = 0.62). Finally, the
antimicrobial, cytotoxic, and epigenetic effects of
Chi-TA-NPs were more pronounced than those of free TA and
the unloaded Chi-NPs. In conclusion, Chi-TA-NPs exhibit
promising potential for reducing microbial growth and
promoting cytotoxicity in liver cancer cells.},
keywords = {Chitosan: chemistry / Chitosan: pharmacology / Humans /
Tannins: chemistry / Tannins: pharmacology / Nanoparticles:
chemistry / Hep G2 Cells / Anti-Infective Agents:
pharmacology / Anti-Infective Agents: chemistry /
Epigenesis, Genetic: drug effects / Candida albicans: drug
effects / Microbial Sensitivity Tests / Antineoplastic
Agents: pharmacology / Antineoplastic Agents: chemistry /
Polyphenols / Antimicrobial effects (Other) / Chitosan
nanoparticles (Other) / Cytotoxicity (Other) / DNA
methylation (Other) / Tannic acid (Other) / Chitosan (NLM
Chemicals) / Tannins (NLM Chemicals) / Anti-Infective Agents
(NLM Chemicals) / Antineoplastic Agents (NLM Chemicals) /
tannic acid (NLM Chemicals) / Polyphenols (NLM Chemicals)},
cin = {B070},
ddc = {600},
cid = {I:(DE-He78)B070-20160331},
pnm = {312 - Funktionelle und strukturelle Genomforschung
(POF4-312)},
pid = {G:(DE-HGF)POF4-312},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:39638815},
doi = {10.1038/s41598-024-80771-x},
url = {https://inrepo02.dkfz.de/record/294828},
}