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@ARTICLE{Gottwald:302804,
author = {W. Gottwald and L. Nagel and J. G. Skinner and M. Grashei
and S. Sühnel and N. Setzer and W. Eisenreich and M. A.
McLean and F. A. Gallagher and J. M. Park and Z. Ahmadova
and M. Gierse and S. Karaali and S. Knecht and I. Schwartz
and I. Heid and G. J. Topping and F. H. A. van Heijster and
F. Schilling$^*$},
title = {{T}emperature dependent chemical shifts of pyruvate and
lactate enable in vivo hyperpolarized 13{C} {MRSI}
thermometry.},
journal = {npj imaging},
volume = {3},
number = {1},
issn = {2948-197X},
address = {[London]},
publisher = {[Nature Publishing Group UK]},
reportid = {DKFZ-2025-01344},
pages = {19},
year = {2025},
abstract = {The chemical shift of many molecules changes with
temperature, which enables non-invasive magnetic resonance
imaging (MRI) thermometry. Hyperpolarization methods
increase the inherently low 13C MR signal. The commonly-used
hyperpolarized probe [1-13C]pyruvate, and its metabolic
product [1-13C]lactate, exhibit temperature and
concentration dependent chemical shift changes that have not
previously been reported. These effects were characterized
at 7 T and 11.7 T in vitro and applied for in vivo
thermometry both preclinically at 7 T and to human data at 3
T. Apparent temperature values from mouse abdomen and brain
were similar to rectally measured temperature. Human brain
and kidney apparent temperatures from 13C MRSI were lower
than known physiological temperatures, suggesting that
additional effects may currently limit the use of this
method for determining absolute temperature in humans. The
temperature dependent chemical shift changes also have
implications for sequence design and for in vitro studies
with hyperpolarized pyruvate.},
cin = {MU01},
cid = {I:(DE-He78)MU01-20160331},
pnm = {899 - ohne Topic (POF4-899)},
pid = {G:(DE-HGF)POF4-899},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:40604117},
pmc = {pmc:PMC12118740},
doi = {10.1038/s44303-025-00081-3},
url = {https://inrepo02.dkfz.de/record/302804},
}