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@ARTICLE{Omer:304880,
author = {E. A. Omer and M. Zhou and W. P. Roos and L. J. Rashan and
H.-H. Fiebig and S. Klauck$^*$ and L. Shan and T. Efferth},
title = {{O}leandrin-mediated suppression of {MELK} induces
apoptosis, autophagy, and ferroptosis in human non-small
cell lung cancer cells.},
journal = {Phytomedicine},
volume = {147},
issn = {0944-7113},
address = {München [u.a.]},
publisher = {Elsevier},
reportid = {DKFZ-2025-01956},
pages = {157173},
year = {2025},
abstract = {Non-small-cell lung cancer NSCLC is the major diagnosed
type of lung cancers in the USA and Europe. It is generally
related to poor prognosis and low rates of survival.
Oleandrin is a cardiac glycoside occurring naturally in
Nerium oleander (Apocynaceae).To explore the potential
therapeutic value of oleandrin against different cancer
types with emphasis on NSCLC.The effect of oleandrin in
inhibiting the growth of different cancer cells was
measured. In addition, oleandrin activity in inhibiting cell
migration, suppression of MELK and inducing different modes
of cell deaths were investigated using in silico, in vitro,
and in vivo methods.Oleandrin showed activity at low
nanomolar level against 17 different types of cancer cells
including NSCLC. Our investigations in A549 cells indicated
that oleandrin is a MELK inhibitor, as it disrupted the
microtubule network and inhibited migration of A549 cells.
Moreover, it induced apoptosis, autophagy, and ferroptosis.
Furthermore, our in vivo data revealed that oleandrin had
significantly decreased tumor growth in a A549 xenograft
zebrafish model in a dose-dependent manner. In silico
analyses revealed that oleandrin bound to the ligand binding
pocket with higher binding affinity than the known inhibitor
MELK-8a. The binding was further confirmed in vitro using
microscale thermophoresis. An ADMET (absorption,
distribution, metabolism, excretion, toxicity) analysis,
together with our in vivo toxicity studies and the previous
clinical studies suggest that oleandrin has an acceptable
safety profile.Oleandrin could potentially have therapeutic
effects for NSCLC patients and possibly for other cancer
types.},
keywords = {Humans / Cardenolides: pharmacology / Carcinoma,
Non-Small-Cell Lung: drug therapy / Animals / Apoptosis:
drug effects / Zebrafish / Lung Neoplasms: drug therapy /
Autophagy: drug effects / Ferroptosis: drug effects / A549
Cells / Cell Movement: drug effects / Cell Line, Tumor /
Antineoplastic Agents, Phytogenic: pharmacology / Xenograft
Model Antitumor Assays / Nerium: chemistry / Cardiac
glycosides (Other) / In vivo (Other) / NSCLC (Other) /
Natural products (Other) / Nerium oleander (Other) /
Phytotherapy (Other) / Programmed cell death (Other) /
Cardenolides (NLM Chemicals) / oleandrin (NLM Chemicals) /
Antineoplastic Agents, Phytogenic (NLM Chemicals)},
cin = {B063},
ddc = {610},
cid = {I:(DE-He78)B063-20160331},
pnm = {312 - Funktionelle und strukturelle Genomforschung
(POF4-312)},
pid = {G:(DE-HGF)POF4-312},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:40916237},
doi = {10.1016/j.phymed.2025.157173},
url = {https://inrepo02.dkfz.de/record/304880},
}