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@ARTICLE{deMaissin:277486,
author = {H. de Maissin$^*$ and P. R. Groß and O. Mohiuddin and M.
Weigt and L. Nagel and M. Herzog and Z. Wang and R.
Willing$^*$ and W. Reichardt and M. Pichotka and L. Heß and
T. Reinheckel$^*$ and H. J. Jessen and R. Zeiser$^*$ and M.
Bock and D. von Elverfeldt and M. Zaitsev and S. Korchak and
S. Glöggler and J.-B. Hövener and E. Y. Chekmenev and F.
Schilling$^*$ and S. Knecht and A. Schmidt$^*$},
title = {{I}n {V}ivo {M}etabolic {I}maging of [1-13{C}]{P}yruvate-d3
{H}yperpolarized {B}y {R}eversible {E}xchange {W}ith
{P}arahydrogen.},
journal = {Angewandte Chemie / International edition},
volume = {62},
number = {36},
issn = {1433-7851},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {DKFZ-2023-01399},
pages = {e202306654},
year = {2023},
note = {2023 Sep 4;62(36):e202306654},
abstract = {Metabolic magnetic resonance imaging (MRI) using
hyperpolarized (HP) pyruvate is becoming a non-invasive
technique for diagnosing, staging, and monitoring response
to treatment in cancer and other diseases. The clinically
established method for producing HP pyruvate, dissolution
dynamic nuclear polarization, however, is rather complex and
slow. Signal Amplification By Reversible Exchange (SABRE) is
an ultra-fast and low-cost method based on fast chemical
exchange. Here, for the first time, we demonstrate not only
in vivo utility, but also metabolic MRI with SABRE. We
present a novel routine to produce aqueous HP
[1-13C]pyruvate-d3 for injection in 6 minutes. The injected
solution was sterile, non-toxic, pH neutral and contained
≈30 mM [1-13C]pyruvate-d3 polarized to $≈11\%$ (residual
250 mM methanol and 20 µM catalyst). It was obtained by
rapid solvent evaporation and metal filtering, which we
detail in this manuscript. This achievement makes HP
pyruvate MRI available to a wide biomedical community for
fast metabolic imaging of living organisms.},
keywords = {SABRE (Other) / hyperpolarization (Other) / metabolic
imaging (Other) / parahydrogen (Other) / pyruvate (Other)},
cin = {FR01 / MU01},
ddc = {540},
cid = {I:(DE-He78)FR01-20160331 / I:(DE-He78)MU01-20160331},
pnm = {899 - ohne Topic (POF4-899)},
pid = {G:(DE-HGF)POF4-899},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:37439488},
doi = {10.1002/anie.202306654},
url = {https://inrepo02.dkfz.de/record/277486},
}