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@ARTICLE{Kritsiligkou:285568,
author = {P. Kritsiligkou$^*$ and K. Bosch$^*$ and T.-K. Shen$^*$ and
M. Meurer$^*$ and M. Knop$^*$ and T. Dick$^*$},
title = {{P}roteome-wide tagging with an {H}2{O}2 biosensor reveals
highly localized and dynamic redox microenvironments.},
journal = {Proceedings of the National Academy of Sciences of the
United States of America},
volume = {120},
number = {48},
issn = {0027-8424},
address = {Washington, DC},
publisher = {National Acad. of Sciences},
reportid = {DKFZ-2023-02434},
pages = {e2314043120},
year = {2023},
note = {DKFZ-ZMBH Alliance / #EA:A160#LA:A160# / 2023 Nov
28;120(48):e2314043120},
abstract = {Hydrogen peroxide (H2O2) sensing and signaling involves the
reversible oxidation of particular thiols on particular
proteins to modulate protein function in a dynamic manner.
H2O2 can be generated from various intracellular sources,
but their identities and relative contributions are often
unknown. To identify endogenous 'hotspots' of H2O2
generation on the scale of individual proteins and protein
complexes, we generated a yeast library in which the H2O2
sensor HyPer7 was fused to the C-terminus of all
protein-coding open reading frames (ORFs). We also generated
a control library in which a redox-insensitive mutant of
HyPer7 (SypHer7) was fused to all ORFs. Both libraries were
screened side-by-side to identify proteins located within
H2O2-generating environments. Screening under a variety of
different metabolic conditions revealed dynamic changes in
H2O2 availability highly specific to individual proteins and
protein complexes. These findings suggest that intracellular
H2O2 generation is much more localized and functionally
differentiated than previously recognized.},
keywords = {genetically encoded probes (Other) / hydrogen peroxide
(Other) / redox regulation (Other) / redox signaling
(Other)},
cin = {A160 / A260},
ddc = {500},
cid = {I:(DE-He78)A160-20160331 / I:(DE-He78)A260-20160331},
pnm = {311 - Zellbiologie und Tumorbiologie (POF4-311)},
pid = {G:(DE-HGF)POF4-311},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:37991942},
doi = {10.1073/pnas.2314043120},
url = {https://inrepo02.dkfz.de/record/285568},
}